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Park, Cheol-Min
Synthetic & Medicinal Chemistry Lab
Research Interests
  • Organic synthesis, medicinal chemistry, chemical biology

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Rhodium(III)-Catalyzed Intramolecular Annulation through C?H Activation: Total Synthesis of (+/-)-Antofine, (+/-)-Septicine, (+/-)-Tylophorine, and Rosettacin

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Title
Rhodium(III)-Catalyzed Intramolecular Annulation through C?H Activation: Total Synthesis of (+/-)-Antofine, (+/-)-Septicine, (+/-)-Tylophorine, and Rosettacin
Author
Xu, XianxiuLiu, YuPark, Cheol-Min
Issue Date
2012
Publisher
WILEY-V C H VERLAG GMBH
Citation
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, v.51, no.37, pp.9372 - 9376
Abstract
Annulation: The efficient synthesis of 3-hydroxyalkyl isoquinolones and 6-hydroxyalkyl 2-pyridones is enabled through the intramolecular annulation of alkyne-tethered hydroxamic esters (see scheme, Cp*= pentamethylcyclopentadienyl). The reaction features high regioselectivity, broad substrate scope, and excellent functional-group tolerance, proceeds under mild reaction conditions with low catalyst loading, and obviates the need for an external oxidant.
URI
https://scholarworks.unist.ac.kr/handle/201301/8538
URL
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=84865841810
DOI
10.1002/anie.201204970
ISSN
1433-7851
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CHM_Journal Papers
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