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Park, Cheol-Min
Synthetic & Medicinal Chemistry Lab
Research Interests
  • Organic synthesis, medicinal chemistry, chemical biology

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Expedient Synthesis of Highly Substituted Pyrroles via Tandem Rearrangement of alpha-Diazo Oxime Ethers

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Title
Expedient Synthesis of Highly Substituted Pyrroles via Tandem Rearrangement of alpha-Diazo Oxime Ethers
Author
Jiang, YaojiaChan, Wei ChuenPark, Cheol-Min
Keywords
2H-Azirines; Oxime ethers; Quaternary centers; Rhodium-catalyzed synthesis
Issue Date
2012-03
Publisher
AMER CHEMICAL SOC
Citation
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, v.134, no.9, pp.4104 - 4107
Abstract
An efficient rhodium-catalyzed synthesis of 2H-azirines and pyrroles has been developed. Novel rearrangement of α-oximino ketenes derived from α-diazo oxime ethers provides 2H-azirines bearing quaternary centers and allows for subsequent rearrangement to highly substituted pyrroles in excellent yields.
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DOI
10.1021/ja300552c
ISSN
0002-7863
Appears in Collections:
PHY_Journal Papers
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