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Jeong, Hu Young
UNIST Central Research Facilities (UCRF)
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  • Soft material characterization such as graphene using a low kV Cs-corrected TEM
  • Insitu-TEM characterization of carbon-based materials using nanofactory STM holder for Li-ion battery application
  • Structural characterization of mesoporous materials using SEM & TEM
  • Interface analysis between various oxides and metals through Cs-corrected (S)TEM
  • Resistive switching mechanism of graphene oxide thin films for RRAM application

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P-type electrical contacts for 2D transition-metal dichalcogenides

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Title
P-type electrical contacts for 2D transition-metal dichalcogenides
Author
Wang, YanKim, Jong ChanLi, YangMa, Kyung YeolHong, SeokmoKim, MinsuShin, Hyeon SukJeong, Hu YoungChhowalla, Manish
Issue Date
2022-08
Publisher
NATURE PORTFOLIO
Citation
NATURE, v.610, pp.61 - 66
Abstract
Digital logic circuits are based on complementary pairs of n- and p-type field effect transistors (FETs) via complementary metal oxide semiconductor technology. In three-dimensional (3D) or bulk semiconductors, substitutional doping of acceptor or donor impurities is used to achieve p- and n-type FETs. However, the controllable p-type doping of low-dimensional semiconductors such astwo-dimensional (2D) transition-metal dichalcogenides (TMDs) has proved to be challenging. Although it is possible to achieve high-quality, low-resistance n-type van der Waals (vdW) contacts on 2D TMDs(1-)(5), obtaining p-type devices by evaporating high-work-function metals onto 2D TMDs has not been realized so far. Here we report high-performance p-type devices on single- and few-layered molybdenum disulfide and tungsten diselenide based on industry-compatible electron beam evaporation of high-work-function metals such as palladium and platinum. Using atomic resolution imaging and spectroscopy, we demonstrate near-ideal vdW interfaces without chemical interactions between the 2D TMDs and 3D metals. Electronic-transport measurements reveal that the Fermi level is unpinned and p-type FETs based on vdW contacts exhibit low contact resistance of 3.3 k Omega mu m, high mobility values of approximately 190 cm(2) V(-1)s(-1) at room temperature, saturation currents in excess of 10(-5) A mu m(-1) and an on/off ratio of 10(7). We also demonstrate an ultra-thin photovoltaic cell based on n- and p-type vdW contacts with an open circuit voltage of 0.6 V and a power conversion efficiency of 0.82%.
URI
https://scholarworks.unist.ac.kr/handle/201301/59590
DOI
10.1038/s41586-022-05134-w
ISSN
0028-0836
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