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Park, Cheol-Min
Synthetic & Medicinal Chemistry Lab
Research Interests
  • Organic synthesis, medicinal chemistry, chemical biology

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Three-Component Synthesis of Quinolines Based on Radical Cascade Visible-Light Photoredox Catalysis

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Title
Three-Component Synthesis of Quinolines Based on Radical Cascade Visible-Light Photoredox Catalysis
Author
Cjoi, Jun-HoPark, Cheol-Min
Issue Date
2018-09
Publisher
WILEY-V C H VERLAG GMBH
Citation
ADVANCED SYNTHESIS & CATALYSIS, v.360, no.18, pp.3553 - 3562
Abstract
Synthesis of highly substituted quinolines has been developed based on three‐component radical cascade based on visible‐light photoredox catalysis. This tandem coupling reaction has been coordinated to proceed with high chemoselectivity based on the differential electronic properties of coupling partners. Subjection of electron‐rich β‐aminoacrylates with electron‐deficient halides and alkenes to the optimized conditions leads to the formation of quinolines in good yields after in situ oxidation of tetrahydroquinolines. Detailed mechanistic studies which reveal an unexpected reaction pathway is described.
URI
https://scholarworks.unist.ac.kr/handle/201301/25028
URL
https://onlinelibrary.wiley.com/doi/abs/10.1002/adsc.201800734
DOI
10.1002/adsc.201800734
ISSN
1615-4150
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PHY_Journal Papers
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