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Schultz, Thomas
CRASY (Correlated Rotational Alignment Spectroscopy)
Research Interests
  • Correlated spectroscopy
  • Ultrafast spectroscopy
  • High-resolution spectroscopy
  • Photochemistry

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CRASY: Mass- or Electron-Correlated Rotational Alignment Spectroscopy

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Title
CRASY: Mass- or Electron-Correlated Rotational Alignment Spectroscopy
Author
Schroeter, ChristianKosma, KyriakiSchultz, Thomas
Issue Date
2011-08
Publisher
AMER ASSOC ADVANCEMENT SCIENCE
Citation
SCIENCE, v.333, no.6045, pp.1011 - 1015
Abstract
Rotational spectra have traditionally been measured without a concurrent means of differentiating the molecular constituents of the sample. Here, we present an all-optical multipulse experiment that allows the correlated measurement of rotational and mass or photoelectron spectra by combining Fourier transform rotational coherence spectroscopy with resonance-enhanced multiphoton ionization. We demonstrate the power of this method with the determination of ground-state rotational constants and fragmentation channels for 10 different isotopes in a natural carbon disulfide sample. Three of the reported rotational constants were previously inaccessible by conventional spectroscopic techniques.
URI
https://scholarworks.unist.ac.kr/handle/201301/6234
URL
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=80051890881
DOI
10.1126/science.1204352
ISSN
0036-8075
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CHM_Journal Papers
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