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- Schultz, Thomas
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Solvated electrons at the water-air interface: surface versus bulk signal in low kinetic energy photoelectron spectroscopy
- Author(s)
- Buchner, Franziska, Schultz, Thomas, Luebcke, Andrea
- Issued Date
- 2012-04
- Citation
- PHYSICAL CHEMISTRY CHEMICAL PHYSICS, v.14, no.16, pp.5837 - 5842
- Abstract
- Time-resolved photoelectron spectroscopy at low kinetic energies (less than or similar to 5 eV) is applied to dilute iodide solutions with different surface and bulk contributions. The results indicate a pronounced surface sensitivity. Signals assigned to solvated electrons near the liquid surface decay rapidly on a sub-ps timescale. In contrast to the literature, a long-lived surface solvated electron at 1.6 eV binding energy is not observed.
- Publisher
- ROYAL SOC CHEMISTRY
- ISSN
- 1463-9076
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