Geostationary satellite-derived ground-level particulate matter concentrations using real-time machine learning in Northeast Asia

Abstract

Rapid economic growth, industrialization, and urbanization have caused frequent air pollution events in East Asia over the last few decades. Recently, aerosol data from geostationary satellite sensors have been used to monitor ground-level particulate matter (PM) concentrations hourly. However, many studies have focused on using historical datasets to develop PM estimation models, often decreasing their predictability for unseen data in new days. To mitigate this problem, this study proposes a novel real-time learning (RTL) approach to estimate PM with aerodynamic diameters of < 10 mu m (PM10) and < 2.5 mu m (PM2.5) using hourly aerosol data from the Geostationary Ocean Color Imager (GOCI) and numerical model outputs for daytime conditions over Northeast Asia. Three schemes with different weighting strategies were evaluated using 10-fold cross-validation (CV). The RTL models, which considered both concentration and time as weighting factors (i.e., Scheme 3) yielded consistent improvement for 10-fold CV performance on both hourly and monthly scales. The real-time calibration results for PM10 and PM2.5 were R-2 = 0.97 and 0.96, and relative root mean square error (rRMSE) = 12.1% and 12.0%, respectively, and the 10-fold CV results for PM10 and PM2.5 were R-2 = 0.73 and 0.69 and rRMSE = 41.8% and 39.6%, respectively. These results were superior to results from the offline models in previous studies, which were based on historical data on an hourly scale. Moreover, we estimated PM concentrations in the ocean without using land-based variables, and clearly demonstrated the PM transport over time. Because the proposed models are based on the RTL approach, the density of in-situ monitoring sites could be a major uncertainty factor. This study identified that a high error occurred in low-density areas, whereas a low error occurred in high density areas. The proposed approach can be operated to monitor ground-level PM concentrations in real-time with uncertainty analysis to ensure optimal results.