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Lim, Hankwon
Sustainable Process Analysis, Design, and Engineering (SPADE)
Research Interests
  • Process analysis, Process design, Techno-economic analysis, Separation process, Reaction engineering, Computational fluid dynamics, Membrane reactor, H2 energy, Water electrolysis, Vanadium redox flow battery, Greenhouse gas reduction

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CFD simulation of methane steam reforming in a membrane reactor: Performance characteristics over range of operating window

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Title
CFD simulation of methane steam reforming in a membrane reactor: Performance characteristics over range of operating window
Author
Upadhyay, MukeshLee, HyunjunKim, AyeonLee, Sang-hunLim, Hankwon
Issue Date
2021-08
Publisher
PERGAMON-ELSEVIER SCIENCE LTD
Citation
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, v.46, no.59, pp.30402 - 30411
Abstract
Methane steam reforming is the most widely used pathway for hydrogen production. In this context, the use of a fixed bed catalytic reactor with a hydrogen-selective membrane is one of the most promising technologies to produce high purity hydrogen gas. In this work, the membrane reactor three-dimensional computational fluid dynamic (CFD) model was developed to investigate the performance. In this model, methane steam reforming global kinetic model has been coupled with the CFD model using User-Defined Function (UDF). Whereas, hydrogen permeation across the membrane is implemented by introducing source and sink formulation. The CFD simulation results were compared to the experimental data, where the developed model successfully captured the experimentally observed trends. We studied the influence of the various operating parameters, as temperature, steam to carbon ratio, sweep gas flow configuration and space velocity on the overall performance. The main observation and attained optimal operation windows from the study was discussed to provide insight into the factors affecting the overall performance. (c) 2021 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
URI
https://scholarworks.unist.ac.kr/handle/201301/53964
URL
https://www.sciencedirect.com/science/article/pii/S0360319921024617?via%3Dihub
DOI
10.1016/j.ijhydene.2021.06.178
ISSN
0360-3199
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