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Lee, Dong Woog
Interfacial Physics and Chemistry Laboratory
Research Interests
  • Bio/Bio-inspired adhesion and lubrication, friction of skin and sensory perception, wetting behavior of various surfaces, surface physics and chemistry of low-dimensional materials

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Adaptive amphiphilic interaction mechanism of hydroxypropyl methylcellulose in water

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dc.contributor.author Lim, Chanoong ko
dc.contributor.author Song, Young Hoon ko
dc.contributor.author Song, Yoojung ko
dc.contributor.author Seo, Jeong Hyun ko
dc.contributor.author Hwang, Dong Soo ko
dc.contributor.author Lee, Dong Woog ko
dc.date.available 2021-07-22T08:15:05Z -
dc.date.created 2021-07-20 ko
dc.date.issued 2021-11 ko
dc.identifier.citation APPLIED SURFACE SCIENCE, v.565, pp.150535 ko
dc.identifier.issn 0169-4332 ko
dc.identifier.uri https://scholarworks.unist.ac.kr/handle/201301/53244 -
dc.description.abstract Hydroxypropyl methylcellulose (HPMC), an FDA-approved water-soluble cellulose derivative, has been used in various wet-adhesion applications in construction products, paints, and drug delivery for 70 years. Despite the various applications, its adhesion mechanism in water has not been elucidated. Here, we measure the adhesion characteristics of HPMC against itself, hydrophilic and hydrophobic surfaces as a function of temperature using a surface forces apparatus (SFA) in water. The results show that HPMC adheres strongly to all tested surfaces, regardless of hydrophobicity. The adhesive strength of HPMC increases with temperature because of entropydriven hydrophobic interactions and is comparable to or exceeds the wet-adhesion strength of most biological adhesives, including those of mussels and cephalopods. In addition, the elevated temperature induces swelling in HPMC layer, resulting in the exposure of more hydrogen bonding sites, thereby increasing adhesion with the hydrophilic surface. The bulk compression test of the HPMC-silica composite material is consistent with the SFA data and indicates that the water content and temperature are critical variables for the adhesion of HPMC to inorganic surfaces regardless of hydrophobicity. Because adhesive and coating technologies have shifted toward environmentally-friendly systems, these results provide a basis for the fabrication of organic solvent-free HPMCbased composites for future applications. ko
dc.language 영어 ko
dc.publisher ELSEVIER ko
dc.title Adaptive amphiphilic interaction mechanism of hydroxypropyl methylcellulose in water ko
dc.type ARTICLE ko
dc.identifier.scopusid 2-s2.0-85109677586 ko
dc.identifier.wosid 000681173500005 ko
dc.type.rims ART ko
dc.identifier.doi 10.1016/j.apsusc.2021.150535 ko
dc.identifier.url https://www.sciencedirect.com/science/article/pii/S0169433221016056?via%3Dihub ko
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