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Cho, Jaephil
Nano Energy Storage Material Lab.
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Magnesium(II) bis(trifluoromethane sulfonyl) imide-based electrolytes with wide electrochemical windows for rechargeable magnesium batteries

Author(s)
Ha, Se-YoungLee, Yong-WonWoo, Sang WonKoo, BonjaeKim, Jeom-SooCho, JaephilLee, Kyu TaeChoi, Nam-Soon
Issued Date
2014-03
DOI
10.1021/am405619v
URI
https://scholarworks.unist.ac.kr/handle/201301/4302
Fulltext
http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=84896956339
Citation
ACS APPLIED MATERIALS & INTERFACES, v.6, no.6, pp.4063 - 4073
Abstract
We present a promising electrolyte candidate, Mg(TFSI)2 dissolved in glyme/diglyme, for future design of advanced magnesium (Mg) batteries. This electrolyte shows high anodic stability on an aluminum current collector and allows Mg stripping at the Mg electrode and Mg deposition on the stainless steel or the copper electrode. It is clearly shown that nondendritic and agglomerated Mg secondary particles composed of ca. 50 nm primary particles alleviating safety concern are formed in glyme/diglyme with 0.3 M Mg(TFSI) 2 at a high rate of 1C. Moreover, a Mg(TFSI)2-based electrolyte presents the compatibility toward a Chevrel phase Mo 6S8, a radical polymer charged up to a high voltage of 3.4 V versus Mg/Mg2+ and a carbon-sulfur composite as cathodes.
Publisher
AMER CHEMICAL SOC
ISSN
1944-8244

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