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Redox Cofactor from Biological Energy Transduction as Molecularly Tunable Energy-Storage Compound

Author(s)
Lee, Minah, Hong, Jihyun, Seo, Dong-Hwa, Nam, Dong Heon, Nam, Ki Tae, Kang, Kisuk, Park, Chan Beum
Issued Date
2013-08
DOI
10.1002/anie.201301850
URI
https://scholarworks.unist.ac.kr/handle/201301/30541
Fulltext
https://onlinelibrary.wiley.com/doi/full/10.1002/anie.201301850
Citation
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, v.52, no.32, pp.8322 - 8328
Abstract
Flavin Battery: Flavins are used as a molecularly tunable cathode material that reversibly reacts with two lithium ions and two electrons per formula unit. Combined ex situ analyses and DFT calculations reveal that the redox reaction occurs using two successive single‐electron transfer steps at nitrogen atoms of the diazabutadiene motif.
Publisher
John Wiley & Sons Ltd.
ISSN
1433-7851
Keyword (Author)
flavins, lithium battery, organic electrodes, bioenergetics, biomimetics
Keyword
GAUSSIAN-BASIS SETS, LI-ION BATTERIES, ELECTRON-TRANSFER, FLAVOENZYME ACTIVITY, MODEL SYSTEMS, ATOMS LI, X-RAY, RIBOFLAVIN, SPECTRA, REDUCTION

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