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DC Field | Value | Language |
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dc.citation.number | 39 | - |
dc.citation.startPage | 1703026 | - |
dc.citation.title | ADVANCED MATERIALS | - |
dc.citation.volume | 29 | - |
dc.contributor.author | Seo, Sungbaek | - |
dc.contributor.author | Lee, Dong Woog | - |
dc.contributor.author | Ahn, Jin Soo | - |
dc.contributor.author | Cunha, Keila | - |
dc.contributor.author | Filippidi, Emmanouela | - |
dc.contributor.author | Ju, Sung Won | - |
dc.contributor.author | Shin, Eeseul | - |
dc.contributor.author | Kim, Byeong-Su | - |
dc.contributor.author | Levine, Zachary A. | - |
dc.contributor.author | Lins, Roberto D. | - |
dc.contributor.author | Israelachvili, Jacob N. | - |
dc.contributor.author | Waite, J. Herbert | - |
dc.contributor.author | Valentine, Megan T. | - |
dc.contributor.author | Shea, Joan Emma | - |
dc.contributor.author | Ahn, B. Kollbe | - |
dc.date.accessioned | 2023-12-21T21:41:15Z | - |
dc.date.available | 2023-12-21T21:41:15Z | - |
dc.date.created | 2017-10-30 | - |
dc.date.issued | 2017-10 | - |
dc.description.abstract | Marine mussels use catechol-rich interfacial mussel foot proteins (mfps) as primers that attach to mineral surfaces via hydrogen, metal coordination, electrostatic, ionic, or hydrophobic bonds, creating a secondary surface that promotes bonding to the bulk mfps. Inspired by this biological adhesive primer, it is shown that a ≈1 nm thick catecholic single-molecule priming layer increases the adhesion strength of crosslinked polymethacrylate resin on mineral surfaces by up to an order of magnitude when compared with conventional primers such as noncatecholic silane- and phosphate-based grafts. Molecular dynamics simulations confirm that catechol groups anchor to a variety of mineral surfaces and shed light on the binding mode of each molecule. Here, a ≈50% toughness enhancement is achieved in a stiff load-bearing polymer network, demonstrating the utility of mussel-inspired bonding for processing a wide range of polymeric interfaces, including structural, load-bearing materials. | - |
dc.identifier.bibliographicCitation | ADVANCED MATERIALS, v.29, no.39, pp.1703026 | - |
dc.identifier.doi | 10.1002/adma.201703026 | - |
dc.identifier.issn | 0935-9648 | - |
dc.identifier.scopusid | 2-s2.0-85030983838 | - |
dc.identifier.uri | https://scholarworks.unist.ac.kr/handle/201301/22900 | - |
dc.identifier.url | http://onlinelibrary.wiley.com/doi/10.1002/adma.201703026/abstract | - |
dc.identifier.wosid | 000412925600018 | - |
dc.language | 영어 | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.title | Significant Performance Enhancement of Polymer Resins by Bioinspired Dynamic Bonding | - |
dc.type | Article | - |
dc.description.isOpenAccess | FALSE | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter | - |
dc.relation.journalResearchArea | Chemistry; Science & Technology - Other Topics; Materials Science; Physics | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.subject.keywordAuthor | adhesion | - |
dc.subject.keywordAuthor | dynamic bonding | - |
dc.subject.keywordAuthor | mussels | - |
dc.subject.keywordAuthor | primer | - |
dc.subject.keywordAuthor | surfaces | - |
dc.subject.keywordPlus | MUSSEL-INSPIRED ADHESIVES | - |
dc.subject.keywordPlus | SACRIFICIAL BONDS | - |
dc.subject.keywordPlus | FOOT PROTEINS | - |
dc.subject.keywordPlus | SURFACE | - |
dc.subject.keywordPlus | COMPOSITES | - |
dc.subject.keywordPlus | ELASTOMERS | - |
dc.subject.keywordPlus | MIMICKING | - |
dc.subject.keywordPlus | MECHANICS | - |
dc.subject.keywordPlus | CHEMISTRY | - |
dc.subject.keywordPlus | NETWORKS | - |
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