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Lah, Myoung Soo
Frontier Energy Storage Material Lab.
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Templated and template-free fabrication strategies for zero-dimensional hollow MOF superstructures

Author(s)
Kim, HyehyunLah, Myoung Soo
Issued Date
2017-05
DOI
10.1039/c7dt00389g
URI
https://scholarworks.unist.ac.kr/handle/201301/22293
Fulltext
http://pubs.rsc.org/en/Content/ArticleLanding/2017/DT/C7DT00389G#!divAbstract
Citation
DALTON TRANSACTIONS, v.46, no.19, pp.6146 - 6158
Abstract
Various fabrication strategies for hollow metal-organic framework (MOF) superstructures are reviewed and classified using various types of external templates and their properties. Hollow MOF superstructures have also been prepared without external templates, wherein unstable intermediates obtained during reactions convert to the final hollow MOF superstructures. Many hollow MOF superstructures have been fabricated using hard templates. After the core-shell core@ MOF structure was prepared using a hard template, the core was selectively etched to generate a hollow MOF superstructure. Another approach for generating hollow superstructures is to use a solid reactant as a sacrificial template; this method requires no additional etching process. Soft templates such as discontinuous liquid/emulsion droplets and gas bubbles in a continuous soft phase have also been employed to prepare hollow MOF superstructures.
Publisher
ROYAL SOC CHEMISTRY
ISSN
1477-9226
Keyword
METAL-ORGANIC FRAMEWORKSCOORDINATION POLYMER MICROSPHERESSELECTIVE PERMEABILITYINTERFACIAL SYNTHESISINTERIOR SPACECORE-SHELLNANOSPHERESNANOSTRUCTURESEMULSIONNANOPARTICLES

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