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- Seok, Sang Il
- Laboratory for Energy Harvesting Materials and Systems
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Toward Interaction of Sensitizer and Functional Moieties in Hole-Transporting Materials for Efficient Semiconductor-Sensitized Solar Cells
- Author(s)
- Im, Sang Hyuk, Lim, Choong-Sun, Chang, Jeong Ah, Lee, Yong Hui, Maiti, Nilkamal, Kim, Hi-Jung, Nazeeruddin, Md K., Graetzel, Michael, Seok, Sang Il
- Issued Date
- 2011-11
- Citation
- NANO LETTERS, v.11, no.11, pp.4789 - 4793
- Abstract
- Sb(2)S(3)-sensitized mesoporous-TiO(2) solar cells using several conjugated polymers as hole-transporting materials (HTMs) are fabricated. We found that the cell performance was strongly cc rrelated with the chemical interaction at the interface of Sb(2)S(3) as sensitizer and the HTMs through the thiophene moieties, which led to a higher fill factor (FF), open-circuit voltage (V(oc)), and short-circuit current density (J(sc)). With the application of PCPDTBT (poly(2,6-(4,4-bis-(2-ethylhexyl)-4H-cyclopenta[2,1-b;3,4-b']dithiophene)-alt-4,7(2,1,3-benzothiadiazole)) as a HTM in a Sb(2)S(3)-sensitized solar cell, overall power conversion efficiencies of 6.18, 6.57, and 6.53% at 100, 50, and 10% solar irradiation, respectively, were achieved with a metal mask
- Publisher
- AMER CHEMICAL SOC
- ISSN
- 1530-6984
- Keyword (Author)
- Sensitized solar cells, heterojunction solar cells, functional moieties, Sb(2)S(3), mesoporous TiO(2), hole conducting materials
- Keyword
- QUANTUM DOTS, SPECTRA, SB
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