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- Kee, Jung-Min
- Bioorganic and Chembio Lab.
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Studies on oxidopyrylium [5+2] cycloadditions: Toward a general synthetic route to the C12-hydroxy daphnetoxins
- Alternative Title
- Studies on oxidopyrylium [5+2] cycloadditions: Toward a general syntheti c route to the C12-hydroxy daphnetoxins
- Author(s)
- Wender, Paul A., Bi, F. Christopher, Buschmann, Nicole, Gosselin, Francis, Kan, Cindy, Kee, Jung-Min, Ohmura, Hirofumi
- Issued Date
- 2006-11
- Citation
- ORGANIC LETTERS, v.8, no.23, pp.5373 - 5376
- Abstract
- [GRAPHICS] 12-Hydroxydaphnetoxins, members of the structurally fascinating daphnane diterpene family, exhibit a wide range of significant biological activities. A general route to the BC-ring system of 12-hydroxy daphnetoxins is reported based on D-ribose. Depending on the choice of protecting groups and solvent, the oxidopyrylium-alkene [5+2] cycloaddition originating from A provides cycloadduct diastereomer B or C with good to excellent selectivity
- Publisher
- AMER CHEMICAL SOC
- ISSN
- 1523-7060
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