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Lee, Jae Sung
Eco-friendly Catalysis and Energy Lab
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  • Photocatalytic water splitting, artificial photosynthesis, fuel cells, heterogeneous catalysis

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Oxidative carbonylation of phenol to diphenyl carbonate over supported palladium catalysts

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Title
Oxidative carbonylation of phenol to diphenyl carbonate over supported palladium catalysts
Other Titles
Oxidative carbonylation of phenol to diphenyl carbonate over supported palladium catalysts
Author
Song, Ho YoungPark, Eun DuckLee, Jae Sung
Keywords
oxidative carbonylation; phenol; diphenyl carbonate; hydrophobicity; Pd/C
Issue Date
2000-03
Publisher
ELSEVIER SCIENCE BV
Citation
JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL, v.154, no.1-2, pp.243 - 250
Abstract
Oxidative carbonylation of phenol to form diphenyl carbonate (DPC) was investigated in the multi-step electron transfer system containing homogeneous or heterogeneous palladium as the main component. Carbon-supported Pd catalyst showed a better DPC yield than the best homogeneous system with Pd(OAc)(2) for the same amount of palladium. For the supported palladium catalyst, the hydrophobicity of the supports appeared to be critical for high yields of DPC. The palladium remained in the metallic state and dissolution into the reaction solution was, if there was any, negligible. Effects of promoters in carbon-supported Pd catalyst system were also examined. (C) 2000 Elsevier Science B.V. All rights reserved
URI
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DOI
10.1016/S1381-1169(99)00392-1
ISSN
1381-1169
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ECHE_Journal Papers
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