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Author

Lah, Myoung Soo
Nanoporous Materials Lab
Research Interests
  • Metal-Organic Frameworks (MOFs)

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Concomitant Formation of N-Heterocyclic Carbene-Copper Complexes within a Supramolecular Network in the Self-Assembly of Imidazolium Dicarboxylate with Metal Ions

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Title
Concomitant Formation of N-Heterocyclic Carbene-Copper Complexes within a Supramolecular Network in the Self-Assembly of Imidazolium Dicarboxylate with Metal Ions
Author
Chun, JiseulJung, Il GuKim, Hae JinPark, MiraLah, Myoung SooSon, Seung Uk
Keywords
ORGANIC FRAMEWORKS; HYDROGEN STORAGE; COUPLING REACTIONS; CATALYSIS; CHEMISTRY; POLYMERIZATION; EFFICIENT; REAGENTS; BROMIDES; LIGAND
Issue Date
200907
Publisher
AMER CHEMICAL SOC
Citation
INORGANIC CHEMISTRY, v.48, no.14, pp.6353 - 6355
Abstract
A new building block containing an imidazolium salt was synthesized and used for the construction of supramolecular networks with metal ions. We discovered the concomitant formation of the N-heterocyclic carbene-copper complex (CN = 2) in the selfassembly of imidazolium dlcarboxylates and copper nitrates in N, N-dimethylformamide under heating. The proton in the 2 position of the imidazolium salt was abstracted, and CuII was reduced to CuI during the self-assembly process.
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DOI
http://dx.doi.org/10.1021/ic900846s
ISSN
0020-1669
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