Full metadata record
DC Field | Value | Language |
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dc.citation.startPage | 2405664 | - |
dc.citation.title | ADVANCED MATERIALS | - |
dc.contributor.author | Zhai, Qingfeng | - |
dc.contributor.author | Huang, Hetaishan | - |
dc.contributor.author | Lawson, Tom | - |
dc.contributor.author | Xia, Zhenhai | - |
dc.contributor.author | Giusto, Paolo | - |
dc.contributor.author | Antonietti, Markus | - |
dc.contributor.author | Jaroniec, Mietek | - |
dc.contributor.author | Chhowalla, Manish | - |
dc.contributor.author | Baek, Jong-Beom | - |
dc.contributor.author | Liu, Yun | - |
dc.contributor.author | Qiao, Shizhang | - |
dc.contributor.author | Dai, Liming | - |
dc.date.accessioned | 2024-08-12T10:05:13Z | - |
dc.date.available | 2024-08-12T10:05:13Z | - |
dc.date.created | 2024-08-08 | - |
dc.date.issued | 2024-07 | - |
dc.description.abstract | Over the last decade, carbon-based metal-free electrocatalysts (C-MFECs) have become important in electrocatalysis. This field is started thanks to the initial discovery that nitrogen atom doped carbon can function as a metal-free electrode in alkaline fuel cells. A wide variety of metal-free carbon nanomaterials, including 0D carbon dots, 1D carbon nanotubes, 2D graphene, and 3D porous carbons, has demonstrated high electrocatalytic performance across a variety of applications. These include clean energy generation and storage, green chemistry, and environmental remediation. The wide applicability of C-MFECs is facilitated by effective synthetic approaches, e.g., heteroatom doping, and physical/chemical modification. These methods enable the creation of catalysts with electrocatalytic properties useful for sustainable energy transformation and storage (e.g., fuel cells, Zn-air batteries, Li-O2 batteries, dye-sensitized solar cells), green chemical production (e.g., H2O2, NH3, and urea), and environmental remediation (e.g., wastewater treatment, and CO2 conversion). Furthermore, significant advances in the theoretical study of C-MFECs via advanced computational modeling and machine learning techniques have been achieved, revealing the charge transfer mechanism for rational design and development of highly efficient catalysts. This review offers a timely overview of recent progress in the development of C-MFECs, addressing material syntheses, theoretical advances, potential applications, challenges and future directions. This review comprehensively examines the latest advancements in carbon-based metal-free catalysts for applications in energy, chemical conversions, and environmental remediation. It highlights the related carbon materials, innovative design strategies, and theoretical studies, along with current challenges and forward-looking perspectives on the future directions of this rapidly evolving research field. image | - |
dc.identifier.bibliographicCitation | ADVANCED MATERIALS, pp.2405664 | - |
dc.identifier.doi | 10.1002/adma.202405664 | - |
dc.identifier.issn | 0935-9648 | - |
dc.identifier.scopusid | 2-s2.0-85199359354 | - |
dc.identifier.uri | https://scholarworks.unist.ac.kr/handle/201301/83454 | - |
dc.identifier.wosid | 001275488300001 | - |
dc.language | 영어 | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.title | Recent Advances on Carbon-Based Metal-Free Electrocatalysts for Energy and Chemical Conversions | - |
dc.type | Article | - |
dc.description.isOpenAccess | TRUE | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter | - |
dc.relation.journalResearchArea | Chemistry; Science & Technology - Other Topics; Materials Science; Physics | - |
dc.type.docType | Review; Early Access | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.subject.keywordAuthor | environmental remediation | - |
dc.subject.keywordAuthor | green chemistry | - |
dc.subject.keywordAuthor | renewable energy | - |
dc.subject.keywordAuthor | carbon nanomaterials | - |
dc.subject.keywordAuthor | catalytic mechanism | - |
dc.subject.keywordAuthor | electrocatalyst | - |
dc.subject.keywordPlus | NITROGEN-DOPED CARBON | - |
dc.subject.keywordPlus | SENSITIZED SOLAR-CELLS | - |
dc.subject.keywordPlus | OXYGEN REDUCTION REACTION | - |
dc.subject.keywordPlus | GRAPHENE QUANTUM DOTS | - |
dc.subject.keywordPlus | HYDROGEN-PEROXIDE | - |
dc.subject.keywordPlus | HOLEY-GRAPHENE | - |
dc.subject.keywordPlus | ELECTROCHEMICAL SYNTHESIS | - |
dc.subject.keywordPlus | CHARGE-TRANSFER | - |
dc.subject.keywordPlus | FREE CATALYSTS | - |
dc.subject.keywordPlus | EFFICIENT | - |
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