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dc.citation.endPage 4 -
dc.citation.number 3 -
dc.citation.startPage 1 -
dc.citation.title PHYSICAL REVIEW LETTERS -
dc.citation.volume 99 -
dc.contributor.author Strasfeld, David B. -
dc.contributor.author Shim, Sang-Hee -
dc.contributor.author Zanni, Martin T. -
dc.date.accessioned 2023-12-22T09:12:35Z -
dc.date.available 2023-12-22T09:12:35Z -
dc.date.created 2014-10-13 -
dc.date.issued 2007-07 -
dc.description.abstract We report selective population of the excited vibrational levels of the T1u CO-stretching mode in W(CO)6 using phase-tailored, femtosecond mid-IR (5.2μm, 1923cm-1) pulses. An evolutionary algorithm was used to optimize specific vibrational populations. Stimulated emission peaks, indicative of population inversion, could be induced. Systematic truncation of each optimized pulse allowed for increased understanding of the excitation mechanism. The pulses and techniques developed herein will have broad applications in controlling ground state chemistry and enhancing vibrational spectroscopies. -
dc.identifier.bibliographicCitation PHYSICAL REVIEW LETTERS, v.99, no.3, pp.1 - 4 -
dc.identifier.doi 10.1103/PhysRevLett.99.038102 -
dc.identifier.issn 0031-9007 -
dc.identifier.scopusid 2-s2.0-34547169968 -
dc.identifier.uri https://scholarworks.unist.ac.kr/handle/201301/7153 -
dc.identifier.url http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=34547169968 -
dc.identifier.wosid 000248194700062 -
dc.language 영어 -
dc.publisher AMER PHYSICAL SOC -
dc.title Controlling vibrational excitation with shaped mid-IR pulses -
dc.type Article -
dc.description.journalRegisteredClass scopus -
dc.subject.keywordPlus DYNAMICS -
dc.subject.keywordPlus SPECTROSCOPY -
dc.subject.keywordPlus PHASE -
dc.subject.keywordPlus RELAXATION -
dc.subject.keywordPlus SCATTERING -
dc.subject.keywordPlus MOLECULES -

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