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Schultz, Thomas
CRASY (Correlated Rotational Alignment Spectroscopy)
Research Interests
  • Correlated spectroscopy
  • Ultrafast spectroscopy
  • High-resolution spectroscopy
  • Photochemistry


Role of alkali cations for the excited state dynamics of liquid water near the surface

DC Field Value Language Buchner, Franziska ko Ritze, Hans-Hermann ko Beutler, Marcus ko Schultz, Thomas ko Hertel, Ingolf V. ko Luebcke, Andrea ko 2014-09-23T07:00:22Z - 2014-09-19 ko 2012-07 ko
dc.identifier.citation JOURNAL OF CHEMICAL PHYSICS, v.137, no.2, pp.024503 ko
dc.identifier.issn 0021-9606 ko
dc.identifier.uri -
dc.description.abstract Time-resolved liquid jet photoelectron spectroscopy was used to explore the excited state dynamics at the liquid water surface in the presence of alkali cations. The data were evaluated with the help of ab initio calculations on alkali-water clusters and an extension of these results on the basis of the dielectric continuum model: 160nm, sub-20fs vacuum ultraviolet pulses excite water molecules in the solvent shell of Na + or K + cations and evolve into a transient hydrated complex of alkali-ion and electron. The vertical ionization energy of this transient is about 2.5eV, significantly smaller than that of the solvated electron. ⓒ 2012 American Institute of Physics. ko
dc.description.statementofresponsibility open -
dc.language 영어 ko
dc.publisher AMER INST PHYSICS ko
dc.title Role of alkali cations for the excited state dynamics of liquid water near the surface ko
dc.type ARTICLE ko
dc.identifier.scopusid 2-s2.0-84863936067 ko
dc.identifier.wosid 000306361000024 ko
dc.type.rims ART ko
dc.description.wostc 1 *
dc.description.scopustc 1 * 2015-05-06 * 2014-09-19 *
dc.identifier.doi 10.1063/1.4732582 ko
dc.identifier.url ko
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