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DC Field | Value | Language |
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dc.citation.endPage | 13315 | - |
dc.citation.number | 11 | - |
dc.citation.startPage | 13307 | - |
dc.citation.title | ACS APPLIED ENERGY MATERIALS | - |
dc.citation.volume | 4 | - |
dc.contributor.author | Zhan, Tao | - |
dc.contributor.author | Yang, Mingqun | - |
dc.contributor.author | Cai, Ping | - |
dc.contributor.author | Oh, Jiyeon | - |
dc.contributor.author | Yuan, Xiyue | - |
dc.contributor.author | Wu, Baoqi | - |
dc.contributor.author | Pan, Langheng | - |
dc.contributor.author | Zhao, Yanfei | - |
dc.contributor.author | Yang, Changduk | - |
dc.contributor.author | Duan, Chunhui | - |
dc.contributor.author | Huang, Fei | - |
dc.contributor.author | Cao, Yong | - |
dc.date.accessioned | 2023-12-21T15:07:12Z | - |
dc.date.available | 2023-12-21T15:07:12Z | - |
dc.date.created | 2021-12-23 | - |
dc.date.issued | 2021-11 | - |
dc.description.abstract | A sequentially deposited (SD) active layer with bulk-heterojunction (BHJ) like morphology is developed by utilizing a naphthalenediimide-based polymer acceptor PTzNDI-T with a strong interchain interaction and low solubility and a well-soluble polymer donor J52-Cl. The SD active layer is prepared by first depositing PTzNDI-T solution and then depositing J52-Cl solution without any post-treatments, and a traditional blend-cast (BC) active layer is cast from the blend solution of J52-Cl:PTzNDI-T. Both the conventional and inverted all-polymer solar cells (all-PSCs) with the BC active layer present nearly no photovoltaic performance. In contrast, based on the SD active layer, not only do the inverted all-PSCs show a dramatically increased PCE of 6.08% but the conventional all-PSCs with the same deposition sequence also exhibit a similarly high PCE of 6.29%. Notably, the SD active layer shows BHJ-like morphology with well-distributed donor and acceptor phases and thus offers a similarly high photovoltaic performance in conventional and inverted all-PSCs with the same deposition sequence of polymer acceptor and donor, which is the first report of SD all-PSCs. These results provide different insight to the SD active layer for high-performance all-PSCs. | - |
dc.identifier.bibliographicCitation | ACS APPLIED ENERGY MATERIALS, v.4, no.11, pp.13307 - 13315 | - |
dc.identifier.doi | 10.1021/acsaem.1c02983 | - |
dc.identifier.issn | 2574-0962 | - |
dc.identifier.scopusid | 2-s2.0-85119415304 | - |
dc.identifier.uri | https://scholarworks.unist.ac.kr/handle/201301/55329 | - |
dc.identifier.url | https://pubs.acs.org/doi/10.1021/acsaem.1c02983 | - |
dc.identifier.wosid | 000734173500004 | - |
dc.language | 영어 | - |
dc.publisher | AMER CHEMICAL SOC | - |
dc.title | Sequentially Deposited Active Layer with Bulk-Heterojunction-like Morphology for Efficient Conventional and Inverted All-Polymer Solar Cells | - |
dc.type | Article | - |
dc.description.isOpenAccess | FALSE | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Physical;Energy & Fuels;Materials Science, Multidisciplinary | - |
dc.relation.journalResearchArea | Chemistry;Energy & Fuels;Materials Science | - |
dc.type.docType | Article | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.subject.keywordAuthor | all-polymer solar cells | - |
dc.subject.keywordAuthor | bulk-heterojunction morphology | - |
dc.subject.keywordAuthor | photovoltaic performance | - |
dc.subject.keywordAuthor | sequentially deposited active layer | - |
dc.subject.keywordAuthor | vertical composition distribution | - |
dc.subject.keywordPlus | HIGH V-OC | - |
dc.subject.keywordPlus | ERA | - |
dc.subject.keywordPlus | ACCEPTORS | - |
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