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DC Field | Value | Language |
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dc.citation.number | 38 | - |
dc.citation.startPage | 2101813 | - |
dc.citation.title | ADVANCED ENERGY MATERIALS | - |
dc.citation.volume | 11 | - |
dc.contributor.author | Oh, Kyeong-Seok | - |
dc.contributor.author | Kim, Jung-Hui | - |
dc.contributor.author | Kim, Se-Hee | - |
dc.contributor.author | Oh, Dongrak | - |
dc.contributor.author | Han, Sun-Phil | - |
dc.contributor.author | Jung, Kwangeun | - |
dc.contributor.author | Wang, Zhuyi | - |
dc.contributor.author | Shi, Liyi | - |
dc.contributor.author | Su, Yongxiang | - |
dc.contributor.author | Yim, Taeeun | - |
dc.contributor.author | Yuan, Shuai | - |
dc.contributor.author | Lee, Sang-Young | - |
dc.date.accessioned | 2023-12-21T15:12:33Z | - |
dc.date.available | 2023-12-21T15:12:33Z | - |
dc.date.created | 2021-08-23 | - |
dc.date.issued | 2021-10 | - |
dc.description.abstract | Despite their potential as post lithium-ion batteries, solid-state Li-metal batteries are struggling with insufficient electrochemical sustainability and ambient operation limitations. These challenges mainly stem from lack of reliable solid-state electrolytes. Here, a new class of single-ion conducting quasi-solid-state soft electrolyte (SICSE) for practical semi-solid Li-metal batteries (SSLMBs) is demonstrated. The SICSE consists of an ion-rectifying compliant skeleton and a nonflammable coordinated electrolyte. Rheology-tuned SICSE pastes, in combination with UV curing-assisted multistage printing, allow fabrication of seamlessly integrated SSLMBs (composed of a Li metal anode and LiNi0.8Co0.1Mn0.1 cathode) without undergoing high-pressure/high-temperature manufacturing steps. The single-ion conducting capability of the SICSE plays a viable role in stabilizing the interfaces with the electrodes. The resulting SSLMB full cell exhibits stable cycling performance and bipolar configurations with tunable voltages and high gravimetric/volumetric energy densities (476 Wh kgcell−1/1102 Wh Lcell−1 at four-stacked cells with 16.656 V) under ambient operating conditions, along with low-temperature performance, mechanical foldability, and nonflammability. | - |
dc.identifier.bibliographicCitation | ADVANCED ENERGY MATERIALS, v.11, no.38, pp.2101813 | - |
dc.identifier.doi | 10.1002/aenm.202101813 | - |
dc.identifier.issn | 1614-6832 | - |
dc.identifier.scopusid | 2-s2.0-85112599231 | - |
dc.identifier.uri | https://scholarworks.unist.ac.kr/handle/201301/53540 | - |
dc.identifier.url | https://onlinelibrary.wiley.com/doi/10.1002/aenm.202101813 | - |
dc.identifier.wosid | 000682724000001 | - |
dc.language | 영어 | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.title | Single-Ion Conducting Soft Electrolytes for Semi-Solid Lithium Metal Batteries Enabling Cell Fabrication and Operation under Ambient Conditions | - |
dc.type | Article | - |
dc.description.isOpenAccess | FALSE | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter | - |
dc.relation.journalResearchArea | Chemistry; Energy & Fuels; Materials Science; Physics | - |
dc.type.docType | Article; Early Access | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.subject.keywordAuthor | ambient operation | - |
dc.subject.keywordAuthor | lithium metal batteries | - |
dc.subject.keywordAuthor | multistage printing | - |
dc.subject.keywordAuthor | single-ion conductors | - |
dc.subject.keywordAuthor | soft electrolytes | - |
dc.subject.keywordPlus | POLYMER ELECTROLYTE | - |
dc.subject.keywordPlus | PERFORMANCE | - |
dc.subject.keywordPlus | INTERFACE | - |
dc.subject.keywordPlus | CATHODE | - |
dc.subject.keywordPlus | COMPATIBILITY | - |
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