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DC Field | Value | Language |
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dc.citation.number | 35 | - |
dc.citation.startPage | 2103850 | - |
dc.citation.title | ADVANCED FUNCTIONAL MATERIALS | - |
dc.citation.volume | 31 | - |
dc.contributor.author | Lee, Donggue | - |
dc.contributor.author | Kim, Hong-, I | - |
dc.contributor.author | Kim, Won-Yeong | - |
dc.contributor.author | Cho, Seok-Kyu | - |
dc.contributor.author | Baek, Kyungeun | - |
dc.contributor.author | Jeong, Kihun | - |
dc.contributor.author | Ahn, David B. | - |
dc.contributor.author | Park, Sodam | - |
dc.contributor.author | Kang, Seok Ju | - |
dc.contributor.author | Lee, Sang-Young | - |
dc.date.accessioned | 2023-12-21T15:37:22Z | - |
dc.date.available | 2023-12-21T15:37:22Z | - |
dc.date.created | 2021-06-26 | - |
dc.date.issued | 2021-08 | - |
dc.description.abstract | Despite the enormous potential of aqueous zinc (Zn)-ion batteries as a cost-competitive and safer power source, their practical applications have been plagued by the chemical/electrochemical instability of Zn anodes with aqueous electrolytes. Here, ionic liquid (IL) skinny gels are reported as a new class of water-repellent ion-conducting protective layers customized for Zn anodes. The IL skinny gel (thickness approximate to 500 nm), consisting of hydrophobic IL solvent, Zn salts, and thiol-ene polymer compliant skeleton, prevents the access of water molecules to Zn anodes while allowing Zn2+ conduction for redox reactions. The IL-gel-skinned Zn anode enables sustainable Zn plating/stripping cyclability under 90% depth of discharge (DODZn) without suffering from water-triggered interfacial parasitic reactions. Driven by these advantageous effects, a Zn-ion full cell (IL-gel-skinned Zn-anode||aqueous-electrolyte-containing MnO2 cathode) exhibits high charge/discharge cycling performance (capacity retention approximate to 95.7% after 600 cycles) that lies beyond those achievable with conventional aqueous Zn-ion battery technologies. | - |
dc.identifier.bibliographicCitation | ADVANCED FUNCTIONAL MATERIALS, v.31, no.35, pp.2103850 | - |
dc.identifier.doi | 10.1002/adfm.202103850 | - |
dc.identifier.issn | 1616-301X | - |
dc.identifier.scopusid | 2-s2.0-85107810805 | - |
dc.identifier.uri | https://scholarworks.unist.ac.kr/handle/201301/53133 | - |
dc.identifier.url | https://onlinelibrary.wiley.com/doi/10.1002/adfm.202103850 | - |
dc.identifier.wosid | 000660429800001 | - |
dc.language | 영어 | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.title | Water-Repellent Ionic Liquid Skinny Gels Customized for Aqueous Zn-Ion Battery Anodes | - |
dc.type | Article | - |
dc.description.isOpenAccess | FALSE | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter | - |
dc.relation.journalResearchArea | Chemistry; Science & Technology - Other Topics; Materials Science; Physics | - |
dc.type.docType | Article; Early Access | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.subject.keywordAuthor | aqueous Zn-ion batteries | - |
dc.subject.keywordAuthor | electrode-customized electrolytes | - |
dc.subject.keywordAuthor | ionic liquid skinny gels | - |
dc.subject.keywordAuthor | water-repellent ion-conducting protective layers | - |
dc.subject.keywordAuthor | Zn anodes | - |
dc.subject.keywordPlus | ZINC-AIR BATTERIES | - |
dc.subject.keywordPlus | ORGANIC FRAMEWORK | - |
dc.subject.keywordPlus | ELECTROLYTES | - |
dc.subject.keywordPlus | BIS(TRIFLUOROMETHANESULFONYL)IMIDE | - |
dc.subject.keywordPlus | STATE | - |
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