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dc.citation.number 28 -
dc.citation.startPage 2102138 -
dc.citation.title ADVANCED FUNCTIONAL MATERIALS -
dc.citation.volume 31 -
dc.contributor.author Li, Xiaobo -
dc.contributor.author Dai, Xinyue -
dc.contributor.author Tang, Deqi -
dc.contributor.author Wang, Xiao -
dc.contributor.author Hong, Jinhua -
dc.contributor.author Chen, Chao -
dc.contributor.author Yang, Yang -
dc.contributor.author Lu, Jiangbo -
dc.contributor.author Zhu, Jianguo -
dc.contributor.author Lei, Zhibin -
dc.contributor.author Suenaga, Kazu -
dc.contributor.author Ding, Feng -
dc.contributor.author Xu, Hua -
dc.date.accessioned 2023-12-21T15:40:32Z -
dc.date.available 2023-12-21T15:40:32Z -
dc.date.created 2021-05-14 -
dc.date.issued 2021-07 -
dc.description.abstract Low-symmetry 2D materials with strong in-plane anisotropy are ideal platforms for building multifunctional optoelectronic devices. However, the random orientations and easy formation of multidomain structures lead to the single-crystal synthesis of these materials remains a big challenge. Herein, for the first time, the orientation-controlled synthesis of ReS2, a typical low-symmetry 2D material, is explored via interface engineering based on the strong interaction between the material and Au substrates with different symmetries. It is revealed that the lattice orientation and growth behavior of ReS2 are closely relevant to the lattice symmetry of Au facets. Single crystal ReS2 domains with two and even one orientations are acquired on the four-fold symmetry Au(001) facet and the two-fold symmetry Au(101) facet, respectively. Combined with density functional theory calculations, it is demonstrated that the synergy of ultra-strong ReS2-Au interfacial coupling and reduction of symmetry of Au facet is critical to realizing its intrinsic anisotropic growth. Furthermore, great enhancement of electrical and photoelectrical performances are acquired on the well-aligned single crystal ReS2 device. The progress achieved in this work provides significant guidance for the controllable synthesis of wafer-scale single crystals of low-symmetry 2D materials for their practical device applications. -
dc.identifier.bibliographicCitation ADVANCED FUNCTIONAL MATERIALS, v.31, no.28, pp.2102138 -
dc.identifier.doi 10.1002/adfm.202102138 -
dc.identifier.issn 1616-301X -
dc.identifier.scopusid 2-s2.0-85104337314 -
dc.identifier.uri https://scholarworks.unist.ac.kr/handle/201301/52920 -
dc.identifier.url https://onlinelibrary.wiley.com/doi/10.1002/adfm.202102138 -
dc.identifier.wosid 000640553500001 -
dc.language 영어 -
dc.publisher WILEY-V C H VERLAG GMBH -
dc.title Realizing the Intrinsic Anisotropic Growth of 1T ' ReS2 on Selected Au(101) Substrate toward Large-Scale Single Crystal Fabrication -
dc.type Article -
dc.description.isOpenAccess FALSE -
dc.relation.journalWebOfScienceCategory Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter -
dc.relation.journalResearchArea Chemistry; Science & Technology - Other Topics; Materials Science; Physics -
dc.type.docType Article; Early Access -
dc.description.journalRegisteredClass scie -
dc.description.journalRegisteredClass scopus -
dc.subject.keywordAuthor ReS -
dc.subject.keywordAuthor (2) -
dc.subject.keywordAuthor single crystal -
dc.subject.keywordAuthor anisotropy -
dc.subject.keywordAuthor low‐ -
dc.subject.keywordAuthor symmetry 2D materials -
dc.subject.keywordAuthor orientation control -

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