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Lee, Jae Sung
Eco-friendly Catalysis and Energy Lab
Research Interests
  • Photocatalytic water splitting, artificial photosynthesis, fuel cells, heterogeneous catalysis

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Photocatalytic synthesis of oxygenated hydrocarbons from diesel fuel for mobile deNOx application

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dc.contributor.author Kim, Jae Yul ko
dc.contributor.author Kim, Yeon Ho ko
dc.contributor.author Han, Suenghoon ko
dc.contributor.author Choi, Sun Hee ko
dc.contributor.author Lee, Jae Sung ko
dc.date.available 2014-04-10T01:57:24Z -
dc.date.created 2013-07-04 ko
dc.date.issued 2013-06 -
dc.identifier.citation JOURNAL OF CATALYSIS, v.302, no., pp.58 - 66 ko
dc.identifier.issn 0021-9517 ko
dc.identifier.uri https://scholarworks.unist.ac.kr/handle/201301/3466 -
dc.identifier.uri http://www.scopus.com/inward/record.url?partnerID=HzOxMe3b&scp=84877084660 ko
dc.description.abstract oxygenated hydrocarbons (OHCs) as an effective nitrogen oxide (NOx) reductant in selective catalytic reduction (SCR) systems. Thus, TiO2-based photocatalysts produced OHCs composed mainly of C-1-C-6 aldehydes under UV irradiation, and TiO2-SiO2 mixed oxide photocatalysts showed higher selectivity and yield to OHCs than pristine TiO2 by diluting contiguous Ti sites and suppressing complete oxidation to CO2. The effects of reaction variables were studied in detail. A novel scheme of NOx after-treatment system for diesel engine exhaust line was proposed involving the new photocatalytic reaction, where on-board photocatalytic partial oxidation of a small amount of diesel fuel produced OHCs that were supplied to the deNOx system as NOx reductant. Although further improvement is needed in the selectivity for OHCs as well as the system operability, the proposed scheme could be a more environment-friendly option than the reduction by urea, currently considered the most promising technology. ko
dc.description.statementofresponsibility close -
dc.language ENG ko
dc.publisher ACADEMIC PRESS INC ELSEVIER SCIENCE ko
dc.subject Photocatalytic partial oxidation ko
dc.subject Oxygenated hydrocarbons ko
dc.subject TiO2&#8211 ko
dc.subject SiO2 mixed oxides ko
dc.subject NOx reduction ko
dc.subject Diesel vehicle ko
dc.title Photocatalytic synthesis of oxygenated hydrocarbons from diesel fuel for mobile deNOx application ko
dc.type ARTICLE ko
dc.identifier.scopusid 2-s2.0-84877084660 ko
dc.identifier.wosid 000319639300007 ko
dc.type.rims ART ko
dc.description.scopustc 1 *
dc.date.scptcdate 2014-07-12 *
dc.identifier.doi 10.1016/j.jcat.2013.03.003 ko
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