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DC Field | Value | Language |
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dc.citation.endPage | 177 | - |
dc.citation.number | 1 | - |
dc.citation.startPage | 173 | - |
dc.citation.title | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | - |
dc.citation.volume | 53 | - |
dc.contributor.author | Zhang, Rui | - |
dc.contributor.author | Walker, David A. | - |
dc.contributor.author | Grzybowski, Bartosz A. | - |
dc.contributor.author | de la Cruz, Monica Olvera | - |
dc.date.accessioned | 2023-12-22T03:07:36Z | - |
dc.date.available | 2023-12-22T03:07:36Z | - |
dc.date.created | 2020-07-13 | - |
dc.date.issued | 2014-01 | - |
dc.description.abstract | Self-replication is a remarkable phenomenon in nature that has fascinated scientists for decades. In a self-replicating system, the original units are attracted to a template, which induce their binding. In equilibrium, the energy required to disassemble the newly assembled copy from the mother template is supplied by thermal energy. The possibility of optimizing self-replication was explored by controlling the frequency at which energy is supplied to the system. A model system inspired by a class of light-switchable colloids was considered where light is used to control the interactions. Conditions under which self-replication can be significantly more effective under non-equilibrium, cyclic energy delivery than under equilibrium constant energy conditions were identified. Optimal self-replication does not require constant energy expenditure. Instead, the proper timing at which energy is delivered to the system is an essential controllable parameter to induce high replication rates. | - |
dc.identifier.bibliographicCitation | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, v.53, no.1, pp.173 - 177 | - |
dc.identifier.doi | 10.1002/anie.201307339 | - |
dc.identifier.issn | 1433-7851 | - |
dc.identifier.scopusid | 2-s2.0-84890938322 | - |
dc.identifier.uri | https://scholarworks.unist.ac.kr/handle/201301/33096 | - |
dc.identifier.url | https://onlinelibrary.wiley.com/doi/full/10.1002/anie.201307339 | - |
dc.identifier.wosid | 000328714900021 | - |
dc.language | 영어 | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.title | Accelerated Self-Replication under Non-Equilibrium, Periodic Energy Delivery | - |
dc.type | Article | - |
dc.description.isOpenAccess | FALSE | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Multidisciplinary | - |
dc.relation.journalResearchArea | Chemistry | - |
dc.type.docType | Article | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.subject.keywordAuthor | colloids | - |
dc.subject.keywordAuthor | kinetic Monte Carlo simulations | - |
dc.subject.keywordAuthor | light switchable systems | - |
dc.subject.keywordAuthor | non-equilibrium | - |
dc.subject.keywordAuthor | self-replication | - |
dc.subject.keywordPlus | REPRODUCING MACHINES | - |
dc.subject.keywordPlus | NANOPARTICLES | - |
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