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Song, Chang-Keun
Air Quality Impact Assessment Research Lab.
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  • Environmental Science

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Numerical Sensitivity Tests of Volatile Organic Compounds Emission to PM2.5 Formation during Heat Wave Period in 2018 in Two Southeast Korean Cities

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dc.contributor.author Yang, Geum-Hee ko
dc.contributor.author Jo, Yu-Jin ko
dc.contributor.author Lee, Hyo-Jung ko
dc.contributor.author Song, Chang-Keun ko
dc.contributor.author Kim, Cheol-Hee ko
dc.date.available 2020-05-08T01:35:20Z -
dc.date.created 2020-05-06 ko
dc.date.issued 2020-04 ko
dc.identifier.citation ATMOSPHERE, v.11, no.4, pp.331 ko
dc.identifier.issn 2073-4433 ko
dc.identifier.uri https://scholarworks.unist.ac.kr/handle/201301/32032 -
dc.description.abstract A record-breaking severe heat wave was recorded in southeast Korea from 11 July to 15 August 2018, and the numerical sensitivity simulations of volatile organic compound (VOC) to secondarily generated particulate matter with diameter of less than 2.5 mu m (PM2.5) concentrations were studied in the Busan and Ulsan metropolitan areas in southeast Korea. A weather research and forecasting (WRF) model coupled with chemistry (WRF-Chem) was employed, and we carried out VOC emission sensitivity simulations to investigate variations in PM2.5 concentrations during the heat wave period that occurred from 11 July to 15 August 2018. In our study, when anthropogenic VOC emissions from the Comprehensive Regional Emissions Inventory for Atmospheric Transport Experiment-2015 (CREATE-2015) inventory were increased by approximately a factor of five in southeast Korea, a better agreement with observations of PM2.5 mass concentrations was simulated, implying an underestimation of anthropogenic VOC emissions over southeast Korea. The simulated secondary organic aerosol (SOA) fraction, in particular, showed greater dominance during high temperature periods such as 19-21 July, 2018, with the SOA fractions of 42.3% (in Busan) and 34.3% (in Ulsan) among a sub-total of seven inorganic and organic components. This is considerably higher than observed annual mean organic carbon (OC) fraction (28.4 +/- 4%) among seven components, indicating the enhancement of secondary organic aerosols induced by photochemical reactions during the heat wave period in both metropolitan areas. The PM2.5 to PM10 ratios were 0.69 and 0.74, on average, during the study period in the two cities. These were also significantly higher than the typical range in those cities, which was 0.5-0.6 in 2018. Our simulations implied that extremely high temperatures with no precipitation are significantly important to the secondary generation of PM2.5 with higher secondary organic aerosol fraction via photochemical reactions in southeastern Korean cities. Other possible relationships between anthropogenic VOC emissions and temperature during the heat wave episode are also discussed in this study. ko
dc.language 영어 ko
dc.publisher MDPI ko
dc.title Numerical Sensitivity Tests of Volatile Organic Compounds Emission to PM2.5 Formation during Heat Wave Period in 2018 in Two Southeast Korean Cities ko
dc.type ARTICLE ko
dc.identifier.scopusid 2-s2.0-85084703932 ko
dc.identifier.wosid 000539492200018 ko
dc.type.rims ART ko
dc.identifier.doi 10.3390/atmos11040331 ko
dc.identifier.url https://www.mdpi.com/2073-4433/11/4/331 ko
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