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Kwak, Sang Kyu
Kyu’s MolSim Lab @ UNIST
Research Interests
  • Molecular modeling and simulation, statistical thermodynamics, molecular physics

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Synergistic effect of quinary molten salts and Ruthenium catalyst for high-power-density Lithium-carbon dioxide cell

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dc.contributor.author Baek, Kyungeun ko
dc.contributor.author Jeon, Woo Cheol ko
dc.contributor.author Woo, Seongho ko
dc.contributor.author Kim, Jin Chul ko
dc.contributor.author Lee, Jun Gyeong ko
dc.contributor.author An, Kwangjin ko
dc.contributor.author Kwak, Sang Kyu ko
dc.contributor.author Kang, Seok Ju ko
dc.date.available 2019-12-26T09:29:40Z -
dc.date.created 2019-12-24 ko
dc.date.issued 2020-01 ko
dc.identifier.citation NATURE COMMUNICATIONS, v.11, no.1, pp.456 ko
dc.identifier.issn 2041-1723 ko
dc.identifier.uri https://scholarworks.unist.ac.kr/handle/201301/30649 -
dc.description.abstract With a recent increase in interest in metal-gas batteries, the lithium-carbon dioxide cell has attracted considerable attention because of its extraordinary carbon dioxide-capture ability during the discharge process and its potential application as a power source for Mars exploration. However, owing to the stable lithium carbonate discharge product, the cell enables operation only at low current densities, which significantly limits the application of lithium-carbon dioxide batteries and effective carbon dioxide-capture cells. Here, we investigate a high-performance lithium-carbon dioxide cell using a quinary molten salt electrolyte and ruthenium nanoparticles on the carbon cathode. The nitrate-based molten salt electrolyte allows us to observe the enhanced carbon dioxide-capture rate and the reduced discharge-charge over-potential gap with that of conventional lithium-carbon dioxide cells. Furthermore, owing to the ruthernium catalyst, the cell sustains its performance over more than 300 cycles at a current density of 10.0Ag(-1) and exhibits a peak power density of 33.4mWcm(-2). Lithium-carbon dioxide cells are challenging due to the sluggish electron transfer in the Lithium carbonate in aprotic electrolyte. Here, the authors report synergistic effect of molten salt electrolyte and Ruthenium catalyst to enhance the electrochemical performance of Lithium-carbon dioxide batteries ko
dc.language 영어 ko
dc.publisher NATURE PUBLISHING GROUP ko
dc.title Synergistic effect of quinary molten salts and Ruthenium catalyst for high-power-density Lithium-carbon dioxide cell ko
dc.type ARTICLE ko
dc.identifier.scopusid 2-s2.0-85078198474 ko
dc.identifier.wosid 000558878300003 ko
dc.type.rims ART ko
dc.identifier.doi 10.1038/s41467-019-14121-1 ko
dc.identifier.url https://www.nature.com/articles/s41467-019-14121-1 ko
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