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- Moon, Hoi Ri
- Functional Inorganic Nanomaterials Lab for Energy
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In situ-generated metal oxide catalyst during CO oxidation reaction transformed from redox-active metal-organic framework-supported palladium nanoparticles
- Author(s)
- Kim, Jin Yeong, Jin, Mingshi, Lee, Kyung Joo, Cheon, Jae Yeong, Joo, Sang Hoon, Kim, Ji Man, Moon, Hoi Ri
- Issued Date
- 2012-08
- Citation
- NANOSCALE RESEARCH LETTERS, v.7, no.1, pp.1 - 8
- Abstract
- The preparation of redox-active metal-organic framework (ra-MOF)-supported Pd nanoparticles (NPs) via the redox couple-driven method is reported, which can yield unprotected metallic NPs at room temperature within 10 min without the use of reducing agents. The Pd@ra-MOF has been exploited as a precursor of an active catalyst for CO oxidation. Under the CO oxidation reaction condition, Pd@ra-MOF is transformed into a PdOx-NiOy/C nanocomposite to generate catalytically active species in situ, and the resultant nanocatalyst shows sustainable activity through synergistic stabilization.
- Publisher
- SPRINGER
- ISSN
- 1556-276X
- Keyword (Author)
- redox reaction, metal-organic framework, CO oxidation, metal oxide, nanoparticle, palladium
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