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Cho, Jaephil
Nano Energy Storage Materials Lab (NESM)
Research Interests
  • Li-ion battery, metal-air battery, redox-flow battery, flexible battery .

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Advances and Prospects of Sulfide All-Solid-State Lithium Batteries via One-to-One Comparison with Conventional Liquid Lithium Ion Batteries

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Title
Advances and Prospects of Sulfide All-Solid-State Lithium Batteries via One-to-One Comparison with Conventional Liquid Lithium Ion Batteries
Author
Lee, HyomyungOh, PilgunKim, JunhyeokCha, HyungyeonChae, SujongLee, SanghanCho, Jaephil
Issue Date
2019-07
Publisher
Wiley-VCH Verlag
Citation
ADVANCED MATERIALS, v.31, no.29, pp.1900376
Abstract
Owing to the safety issue of lithium ion batteries (LIBs) under the harsh operating conditions of electric vehicles and mobile devices, all-solid-state lithium batteries (ASSLBs) that utilize inorganic solid electrolytes are regarded as a secure next-generation battery system. Significant efforts are devoted to developing each component of ASSLBs, such as the solid electrolyte and the active materials, which have led to considerable improvements in their electrochemical properties. Among the various solid electrolytes such as sulfide, polymer, and oxide, the sulfide solid electrolyte is considered as the most promising candidate for commercialization because of its high lithium ion conductivity and mechanical properties. However, the disparity in energy and power density between the current sulfide ASSLBs and conventional LIBs is still wide, owing to a lack of understanding of the battery electrode system. Representative developments of ASSLBs in terms of the sulfide solid electrolyte, active materials, and electrode engineering are presented with emphasis on the current status of their electrochemical performances, compared to those of LIBs. As a rational method to realizing high energy sulfide ASSLBs, the requirements for the sulfide solid electrolytes and active materials are provided along through simple experimental demonstrations. Potential future research directions in the development of commercially viable sulfide ASSLBs are suggested. © 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
URI
https://scholarworks.unist.ac.kr/handle/201301/26879
URL
https://onlinelibrary.wiley.com/doi/full/10.1002/adma.201900376
DOI
10.1002/adma.201900376
ISSN
0935-9648
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