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DC Field | Value | Language |
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dc.citation.endPage | 34 | - |
dc.citation.startPage | 28 | - |
dc.citation.title | ELECTROCHIMICA ACTA | - |
dc.citation.volume | 306 | - |
dc.contributor.author | Kim, Mun Kyoung | - |
dc.contributor.author | Kim, Hyeok Joo | - |
dc.contributor.author | Lim, Hyungseob | - |
dc.contributor.author | Kwon, Youngkook | - |
dc.contributor.author | Jeong, Hyung Mo | - |
dc.date.accessioned | 2023-12-21T19:10:43Z | - |
dc.date.available | 2023-12-21T19:10:43Z | - |
dc.date.created | 2019-04-17 | - |
dc.date.issued | 2019-05 | - |
dc.description.abstract | Conversion of carbon dioxide (CO 2 ) to useful chemicals is considered a potential solution to resolve the climate threat. In this study, a facile metal-organic framework (MOF)-mediated strategy to obtain an efficient electrocatalyst for the synthesis of methane (CH 4 ) is suggested. Cu-based MOF-74 was chosen as the precursor, which was electrochemically reduced to obtain Cu nanoparticles (NPs). The porous structure of the MOF serves as a template for the synthesis of isolated Cu NP clusters with high catalytic activities and high efficiencies for the CH 4 production in the electrochemical CO 2 reduction reaction. The MOF-derived Cu NPs demonstrate high Faradaic efficiency (>50%) for the CH 4 production with suppressed C 2 production, and 2.3-fold higher methanation activity at −1.3 V (vs. RHE) compared to the commercial Cu NPs. | - |
dc.identifier.bibliographicCitation | ELECTROCHIMICA ACTA, v.306, pp.28 - 34 | - |
dc.identifier.doi | 10.1016/j.electacta.2019.03.101 | - |
dc.identifier.issn | 0013-4686 | - |
dc.identifier.scopusid | 2-s2.0-85063621317 | - |
dc.identifier.uri | https://scholarworks.unist.ac.kr/handle/201301/26523 | - |
dc.identifier.url | https://www.sciencedirect.com/science/article/pii/S0013468619305171?via%3Dihub | - |
dc.identifier.wosid | 000464148700004 | - |
dc.language | 영어 | - |
dc.publisher | Elsevier Ltd | - |
dc.title | Metal–organic framework-mediated strategy for enhanced methane production on copper nanoparticles in electrochemical CO 2 reduction | - |
dc.type | Article | - |
dc.description.isOpenAccess | FALSE | - |
dc.type.docType | Article | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.subject.keywordAuthor | CO 2 reduction | - |
dc.subject.keywordAuthor | Copper nanoparticles | - |
dc.subject.keywordAuthor | Copper-based MOFs | - |
dc.subject.keywordAuthor | Electrocatalysts | - |
dc.subject.keywordAuthor | Hydrocarbon production | - |
dc.subject.keywordPlus | Carbon dioxide | - |
dc.subject.keywordPlus | Catalyst activity | - |
dc.subject.keywordPlus | Crystalline materials | - |
dc.subject.keywordPlus | Efficiency | - |
dc.subject.keywordPlus | Electrocatalysts | - |
dc.subject.keywordPlus | Metal nanoparticles | - |
dc.subject.keywordPlus | Methane | - |
dc.subject.keywordPlus | Organometallics | - |
dc.subject.keywordPlus | Reduction | - |
dc.subject.keywordPlus | CO2 reduction | - |
dc.subject.keywordPlus | Copper nanoparticles | - |
dc.subject.keywordPlus | Copper-based | - |
dc.subject.keywordPlus | Cu nano-particles | - |
dc.subject.keywordPlus | Faradaic efficiencies | - |
dc.subject.keywordPlus | Hydrocarbon production | - |
dc.subject.keywordPlus | Metal organic framework | - |
dc.subject.keywordPlus | Methane production | - |
dc.subject.keywordPlus | Copper | - |
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