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DC Field | Value | Language |
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dc.citation.endPage | 634 | - |
dc.citation.startPage | 628 | - |
dc.citation.title | APPLIED SURFACE SCIENCE | - |
dc.citation.volume | 443 | - |
dc.contributor.author | Lee, Deuk Yeon | - |
dc.contributor.author | Choi, Jae Hong | - |
dc.contributor.author | Shin, Jung Chul | - |
dc.contributor.author | Jung, Man Ki | - |
dc.contributor.author | Song, Seok Kyun | - |
dc.contributor.author | Suh, Jung Ki | - |
dc.contributor.author | Lee, Chang Young | - |
dc.date.accessioned | 2023-12-21T20:41:52Z | - |
dc.date.available | 2023-12-21T20:41:52Z | - |
dc.date.created | 2018-04-02 | - |
dc.date.issued | 2018-06 | - |
dc.description.abstract | Compared with wet processes, dry functionalization using plasma is fast, scalable, solvent-free, and thus presents a promising approach for grafting functional groups to powdery nanomaterials. Previous approaches, however, had difficulties in maintaining an intimate sample-plasma contact and achieving uniform functionalization. Here, we demonstrate a plasma reactor equipped with a porous filter electrode that increases both homogeneity and degree of functionalization by capturing and circulating powdery carbon nanotubes (CNTs) via vacuum and gas blowing. Spectroscopic measurements verify that treatment with O2/air plasma generates oxygen-containing groups on the surface of CNTs, with the degree of functionalization readily controlled by varying the circulation number. Gas sensors fabricated using the plasma-treated CNTs confirm alteration of molecular adsorption on the surface of CNTs. A sequential treatment with NH3 plasma following the oxidation pre-treatment results in the functionalization with nitrogen species of up to 3.2 wt%. Our approach requiring no organic solvents not only is cost-effective and environmentally friendly, but also serves as a versatile tool that applies to other powdery micro or nanoscale materials for controlled modification of their surfaces. | - |
dc.identifier.bibliographicCitation | APPLIED SURFACE SCIENCE, v.443, pp.628 - 634 | - |
dc.identifier.doi | 10.1016/j.apsusc.2018.02.194 | - |
dc.identifier.issn | 0169-4332 | - |
dc.identifier.scopusid | 2-s2.0-85043398072 | - |
dc.identifier.uri | https://scholarworks.unist.ac.kr/handle/201301/23910 | - |
dc.identifier.url | https://www.sciencedirect.com/science/article/pii/S016943321830549X?via%3Dihub | - |
dc.identifier.wosid | 000428446300075 | - |
dc.language | 영어 | - |
dc.publisher | ELSEVIER SCIENCE BV | - |
dc.title | Plasma functionalization of powdery nanomaterials using porous filter electrode and sample circulation | - |
dc.type | Article | - |
dc.description.isOpenAccess | FALSE | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter | - |
dc.relation.journalResearchArea | Chemistry; Materials Science; Physics | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.subject.keywordAuthor | Carbon nanotubes | - |
dc.subject.keywordAuthor | Nano-powder | - |
dc.subject.keywordAuthor | Dry functionalization | - |
dc.subject.keywordAuthor | Vacuum filtration | - |
dc.subject.keywordAuthor | Circulating-sample plasma | - |
dc.subject.keywordPlus | WALLED CARBON NANOTUBES | - |
dc.subject.keywordPlus | FLUIDIZED-BED REACTOR | - |
dc.subject.keywordPlus | SURFACE MODIFICATION | - |
dc.subject.keywordPlus | PRESSURE PLASMA | - |
dc.subject.keywordPlus | POLYETHYLENE POWDER | - |
dc.subject.keywordPlus | MICROWAVE PLASMA | - |
dc.subject.keywordPlus | OXYGEN PLASMA | - |
dc.subject.keywordPlus | PENETRATION DEPTH | - |
dc.subject.keywordPlus | POLYMER POWDERS | - |
dc.subject.keywordPlus | COMPOSITE FILM | - |
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