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DC Field | Value | Language |
---|---|---|
dc.citation.number | 12 | - |
dc.citation.startPage | 126803 | - |
dc.citation.title | PHYSICAL REVIEW LETTERS | - |
dc.citation.volume | 102 | - |
dc.contributor.author | Kamenetska, M. | - |
dc.contributor.author | koentopp, M. | - |
dc.contributor.author | Whalley, A. C. | - |
dc.contributor.author | Park, Y. S. | - |
dc.contributor.author | Steigerwald, M. L. | - |
dc.contributor.author | Nuckolls, C. | - |
dc.contributor.author | Hybertsen, M. S. | - |
dc.contributor.author | Venkataraman, L. | - |
dc.date.accessioned | 2023-12-22T08:08:15Z | - |
dc.date.available | 2023-12-22T08:08:15Z | - |
dc.date.created | 2016-07-18 | - |
dc.date.issued | 2009-03 | - |
dc.description.abstract | We analyze the formation and evolution statistics of single-molecule junctions bonded to gold electrodes using amine, methyl sulfide, and dimethyl phosphine link groups by measuring conductance as a function of junction elongation. For each link, the maximum elongation and formation probability increase with molecular length, strongly suggesting that processes other than just metal-molecule bond breakage play a key role in junction evolution under stress. Density functional theory calculations of adiabatic trajectories show sequences of atomic-scale changes in junction structure, including shifts in the attachment point, that account for the long conductance plateau lengths observed | - |
dc.identifier.bibliographicCitation | PHYSICAL REVIEW LETTERS, v.102, no.12, pp.126803 | - |
dc.identifier.doi | 10.1103/PhysRevLett.102.126803 | - |
dc.identifier.issn | 0031-9007 | - |
dc.identifier.scopusid | 2-s2.0-63649150380 | - |
dc.identifier.uri | https://scholarworks.unist.ac.kr/handle/201301/20048 | - |
dc.identifier.url | http://journals.aps.org/prl/abstract/10.1103/PhysRevLett.102.126803 | - |
dc.identifier.wosid | 000264632100051 | - |
dc.language | 영어 | - |
dc.publisher | AMER PHYSICAL SOC | - |
dc.title | Formation and Evolution of Single-Molecule Junctions | - |
dc.type | Article | - |
dc.description.journalRegisteredClass | scopus | - |
dc.subject.keywordPlus | BASIS-SETS | - |
dc.subject.keywordPlus | GOLD ATOMS | - |
dc.subject.keywordPlus | CONDUCTANCE | - |
dc.subject.keywordPlus | TRANSPORT | - |
dc.subject.keywordPlus | CIRCUITS | - |
dc.subject.keywordPlus | CONTACTS | - |
dc.subject.keywordPlus | RN | - |
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