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DC Field | Value | Language |
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dc.citation.endPage | 11829 | - |
dc.citation.number | 12 | - |
dc.citation.startPage | 11820 | - |
dc.citation.title | ACS NANO | - |
dc.citation.volume | 9 | - |
dc.contributor.author | Kim, Jin Hyun | - |
dc.contributor.author | Jo, Yimhyun | - |
dc.contributor.author | Kim, Ju Hun | - |
dc.contributor.author | Jang, Ji-Wook | - |
dc.contributor.author | Kang, Hyun Jun | - |
dc.contributor.author | Lee, Young Hye | - |
dc.contributor.author | Kim, Dong Suk | - |
dc.contributor.author | Jun, Yongseok | - |
dc.contributor.author | Lee, Jae Sung | - |
dc.date.accessioned | 2023-12-22T00:17:54Z | - |
dc.date.available | 2023-12-22T00:17:54Z | - |
dc.date.created | 2016-01-25 | - |
dc.date.issued | 2015-12 | - |
dc.description.abstract | A stand-alone, wireless solar water splitting device without external energy supply has been realized by combining in tandem a CH(3)NH(3)Pbl(3) perovskite single junction solar cell with a cobalt carbonate (Co-Ci)-catalyzed, extrinsic/intrinsic dual-doped BiVO4 (hydrogen-treated and 3 at% Mo-doped). The photoanode recorded one of the highest photoelectrochemical water oxidation activity (4.8 mA/cm(2) at 1.23 V-RHE) under simulated 1 sun illumination. The oxygen evolution Co-Ci co-catalyst showed similar performance to best known cobalt phosphate (Co-Pi) (5.0 mA/cm(2) at 1.23 VRHE) on the same dual-doped BiVO4 photoanode, but with significantly better stability. A tandem artificial-leaf-type device produced stoichiometric hydrogen and oxygen with an average solar-to-hydrogen efficiency of 4.3% (wired), 3.0% (wireless) under simulated 1 sun illumination. Hence, our device based on a D4 tandem photoelectrochemical cell represents a meaningful advancement in performance and cost over the device based on a triple-junction solar cell-electrocatalyst combination | - |
dc.identifier.bibliographicCitation | ACS NANO, v.9, no.12, pp.11820 - 11829 | - |
dc.identifier.doi | 10.1021/acsnano.5b03859 | - |
dc.identifier.issn | 1936-0851 | - |
dc.identifier.scopusid | 2-s2.0-84952362034 | - |
dc.identifier.uri | https://scholarworks.unist.ac.kr/handle/201301/18204 | - |
dc.identifier.url | http://pubs.acs.org/doi/abs/10.1021/acsnano.5b03859 | - |
dc.identifier.wosid | 000367280100031 | - |
dc.language | 영어 | - |
dc.publisher | AMER CHEMICAL SOC | - |
dc.title | Wireless Solar Water Splitting Device with Robust Cobalt-Catalyzed, Dual-Doped BiVO4 Photoanode and Perovskite Solar Cell in Tandem: A Dual Absorber Artificial Leaf | - |
dc.type | Article | - |
dc.description.isOpenAccess | FALSE | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary | - |
dc.relation.journalResearchArea | Chemistry; Science & Technology - Other Topics; Materials Science | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.subject.keywordAuthor | dual doping | - |
dc.subject.keywordAuthor | cobalt carbonate | - |
dc.subject.keywordAuthor | BiVO4 | - |
dc.subject.keywordAuthor | perovskite solar cell | - |
dc.subject.keywordAuthor | tandem cell | - |
dc.subject.keywordAuthor | artificial leaf | - |
dc.subject.keywordPlus | BISMUTH VANADATE PHOTOANODES | - |
dc.subject.keywordPlus | EARTH-ABUNDANT CATALYSTS | - |
dc.subject.keywordPlus | OXYGEN EVOLUTION | - |
dc.subject.keywordPlus | VISIBLE-LIGHT | - |
dc.subject.keywordPlus | HYDROGEN-PRODUCTION | - |
dc.subject.keywordPlus | CHARGE SEPARATION | - |
dc.subject.keywordPlus | MONOCLINIC BIVO4 | - |
dc.subject.keywordPlus | CURRENT STATE | - |
dc.subject.keywordPlus | IN-SITU | - |
dc.subject.keywordPlus | OXIDATION | - |
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