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Schultz, Thomas
CRASY(Correlated Rotational Alignment Spectroscopy)
Research Interests
  • Correlated spectroscopy

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Dynamics of excited-state proton transfer systems via time-resolved photoelectron spectroscopy

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Title
Dynamics of excited-state proton transfer systems via time-resolved photoelectron spectroscopy
Author
Lochbrunner, SSchultz, ThomasSchmitt, MShaffer, JPZgierski, MZStolow, A
Keywords
ULTRAFAST INTERNAL-CONVERSION; ORTHO-HYDROXYACETOPHENONE; ORTHO-HYDROXYBENZALDEHYDE; IONIZATION SPECTROSCOPY; POLYATOMIC-MOLECULES; ELECTRONIC STATES; FEMTOSECOND; 1-HYDROXY-2-ACETONAPHTHONE; FLUORESCENCE; CLUSTERS
Issue Date
200102
Publisher
AMER INST PHYSICS
Citation
JOURNAL OF CHEMICAL PHYSICS, v.114, no.6, pp.2519 - 2522
Abstract
The use of time-resolved photoelectron spectroscopy for analyzing excited state intramolecular proton transfer (ESIPT) and internal conversion dynamics in a model system was investigated. The photoelectron spectra of both the excited state enol and keto tautomers were presented as a function of pump laser wavelength and pump-probe time delay. It was found that the internal conversion dynamics in o-hydroxybenzaldehyde (OHBA) was influenced by interactions with a close-lying nπ* state.
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DOI
http://dx.doi.org/10.1063/1.1345876
ISSN
0021-9606
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SNS_Journal Papers
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