Solution-Shear-Processed Quaterrylene Diimide Thin-Film Transistors Prepared by Pressure-Assisted Thermal Cleavage of Swallow Tails
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- Solution-Shear-Processed Quaterrylene Diimide Thin-Film Transistors Prepared by Pressure-Assisted Thermal Cleavage of Swallow Tails
- Oh, Joon Hak; Lee, Wen-Ya; Noe, Torsten; Chen, Wen-Chang; Koenemann, Martin; Bao, Zhenan
- Diimide; Scalable synthesis; Solution-processing; Thermal cleavage
- Issue Date
- AMER CHEMICAL SOC
- JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, v.133, no.12, pp.4204 - 4207
- A scalable synthesis of swallow-tailed quaterrylene diimides (STQDIs) and a method for the solution processing of sparingly soluble quaterrylene diimide (QDI) thin films are described. The pressure-assisted thermal cleavage of swallow tails yields crystalline QDI layers with electron mobility up to 0.088 cm(2) V(-1) s(-1). The developed method opens up a new route toward the solution processing of higher rylene diimides with poor solubility.
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