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DC Field | Value | Language |
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dc.citation.endPage | 1193 | - |
dc.citation.number | 5 | - |
dc.citation.startPage | 1182 | - |
dc.citation.title | CHEM | - |
dc.citation.volume | 5 | - |
dc.contributor.author | Zhang, Shuchen | - |
dc.contributor.author | Wang, Xiao | - |
dc.contributor.author | Yao, Fengrui | - |
dc.contributor.author | He, Maoshuai | - |
dc.contributor.author | Lin, Dewu | - |
dc.contributor.author | Ma, He | - |
dc.contributor.author | Sun, Yangyong | - |
dc.contributor.author | Zhao, Qiuchen | - |
dc.contributor.author | Liu, Kaihui | - |
dc.contributor.author | Ding, Feng | - |
dc.contributor.author | Zhang, Jin | - |
dc.date.accessioned | 2023-12-21T19:09:54Z | - |
dc.date.available | 2023-12-21T19:09:54Z | - |
dc.date.created | 2019-05-30 | - |
dc.date.issued | 2019-05 | - |
dc.description.abstract | Semiconducting single-walled carbon nanotubes (SWNTs) with controlled chirality (n, m) and band gaps are expected to create a new era of electronics. Here, we report a rational design to enable SWNTs' near-equilibrium nucleation and then grow a new family of semiconducting SWNTs: (n, n - 1) carbon nano-tubes. No metallic SWNTs were observed in similar to 100 samples by reflection optical spectral measurements. Combined with catalyst controlling, we have successfully synthesized both large-diameter (>2 nm) (n, n - 1) SWNTs and single-chirality (10, 9) SWNTs with abundances of 88% and >80%, respectively. Theoretical analysis indicates that the chirality of (n, n) tubes tends to change to (n, n - 1) by kinetically incorporating an energetically preferred pentagon-heptagon pair in the tube wall. This strategy opens up a new route for the growth of SWNT families beyond catalyst design. | - |
dc.identifier.bibliographicCitation | CHEM, v.5, no.5, pp.1182 - 1193 | - |
dc.identifier.doi | 10.1016/j.chempr.2019.02.012 | - |
dc.identifier.issn | 2451-9294 | - |
dc.identifier.scopusid | 2-s2.0-85065046363 | - |
dc.identifier.uri | https://scholarworks.unist.ac.kr/handle/201301/26717 | - |
dc.identifier.url | https://www.sciencedirect.com/science/article/pii/S2451929419300695?via%3Dihub | - |
dc.identifier.wosid | 000467750100013 | - |
dc.language | 영어 | - |
dc.publisher | CELL PRESS | - |
dc.title | Controllable Growth of (n, n - 1) Family of Semiconducting Carbon Nanotubes | - |
dc.type | Article | - |
dc.description.isOpenAccess | FALSE | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Multidisciplinary | - |
dc.relation.journalResearchArea | Chemistry | - |
dc.type.docType | Article | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.subject.keywordAuthor | (n, n − 1) family carbon nanotubes | - |
dc.subject.keywordAuthor | catalyst design | - |
dc.subject.keywordAuthor | controlled CVD growth | - |
dc.subject.keywordAuthor | infrared photodetector | - |
dc.subject.keywordAuthor | SDG11: Sustainable cities and communities | - |
dc.subject.keywordAuthor | semiconducting single-walled carbon nanotubes | - |
dc.subject.keywordPlus | CHIRALITY-SPECIFIC GROWTH | - |
dc.subject.keywordPlus | SELECTIVE SYNTHESIS | - |
dc.subject.keywordPlus | DENSITY | - |
dc.subject.keywordPlus | ARRAYS | - |
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