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- Bae, Sung Chul
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Relaxation kinetics on the first excited singlet state of SO2 from time resolved emission spectra
- Issued Date
- 1997-02
- Citation
- CHEMICAL PHYSICS LETTERS, v.265, no.3-5, pp.385 - 391
- Abstract
- The relaxation kinetics on the first excited singlet state ((1)A(2)) of SO2 have been studied from time-resolved emission spectra in the 300-450 nm region. Two rovibronic levels belonging to the Clements E-band and the (1)A(2)(0,8,1) level, which are located above and below the origin of the B-1(1) state, respectively, were excited to investigate the role of the B-1(1) state on the relaxation kinetics. Direct emissions from the Laser excited rovibronic levels in the (1)A(2) state and direct intersystem crossing between the (1)A(2)(0,8,1) and B-3(1) states were observed and revised relaxation kinetic schemes are proposed.
- Publisher
- ELSEVIER SCIENCE BV
- ISSN
- 0009-2614
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