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Lee, Jae Sung
Eco-friendly Catalysis and Energy Lab
Research Interests
  • Photocatalytic water splitting, artificial photosynthesis, fuel cells, heterogeneous catalysis

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Ultrapermeable Nickel-Cobalt-Manganese/Alumina Inverse Opal as a Coke-Tolerant and Pressure-Drop-Free Catalyst for the Dry Reforming of Methane

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Title
Ultrapermeable Nickel-Cobalt-Manganese/Alumina Inverse Opal as a Coke-Tolerant and Pressure-Drop-Free Catalyst for the Dry Reforming of Methane
Author
Kim, Won YongLee, Byung JunPark, HunminChoi, Yo HanKim, Ju HunLee, Jae Sung
Keywords
dry reforming;  inverse opal structure;  macroporous materials;  nanostructures;  permeability
Issue Date
201805
Publisher
WILEY-V C H VERLAG GMBH
Citation
CHEMCATCHEM, v.10, no.10, pp.2214 - 2218
Abstract
An inverse opal-structured Ni-Co-Mn/Al2O3 catalyst with ultrahigh permeability was prepared by a sol-gel method templated by poly(methyl methacrylate) opal-structured nanospheres. This catalyst exhibited excellent coke tolerance and a negligible reactor pressure drop in the dry reforming of methane. The highly permeable, unique macroporous structure allowed facile mass transport, which not only reduced the amount of coke deposition but also enhanced coke tolerance. Therefore, invariant CO2/CH4 conversions despite substantial coke formation were observed.
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DOI
http://dx.doi.org/10.1002/cctc.201702038
ISSN
1867-3880
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