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DC Field | Value | Language |
---|---|---|
dc.citation.endPage | 5076 | - |
dc.citation.number | 20 | - |
dc.citation.startPage | 5072 | - |
dc.citation.title | PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA | - |
dc.citation.volume | 115 | - |
dc.contributor.author | Schroter, Christian | - |
dc.contributor.author | Lee, Jong Chan | - |
dc.contributor.author | Schultz, Thomas | - |
dc.date.accessioned | 2023-12-21T20:46:12Z | - |
dc.date.available | 2023-12-21T20:46:12Z | - |
dc.date.created | 2018-05-01 | - |
dc.date.issued | 2018-05 | - |
dc.description.abstract | We present mass-correlated rotational alignment spectroscopy, based on the optical excitation of a coherent rotational quantum wave and the observation of temporal wave interferences in a mass spectrometer. Combined electronic and opto-mechanical delays increased the observation time and energy resolution by an order of magnitude compared with preceding time-domain measurements. Rotational transition frequencies were referenced to an external clock for accurate absolute frequency measurements. Rotational Raman spectra for six naturally occurring carbon disulfide isotopologues were resolved with 3 MHz resolution over a spectral range of 500 GHz. Rotational constants were determined with single-kilohertz accuracy, competitive with state-of-the-art frequency domain measurements. | - |
dc.identifier.bibliographicCitation | PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, v.115, no.20, pp.5072 - 5076 | - |
dc.identifier.doi | 10.1073/pnas.1721756115 | - |
dc.identifier.issn | 0027-8424 | - |
dc.identifier.scopusid | 2-s2.0-85046939795 | - |
dc.identifier.uri | https://scholarworks.unist.ac.kr/handle/201301/24012 | - |
dc.identifier.url | http://www.pnas.org/content/115/20/5072 | - |
dc.identifier.wosid | 000432120400034 | - |
dc.language | 영어 | - |
dc.publisher | NATL ACAD SCIENCES | - |
dc.title | Mass-correlated rotational Raman spectra with high resolution, broad bandwidth, and absolute frequency accuracy | - |
dc.type | Article | - |
dc.description.isOpenAccess | FALSE | - |
dc.relation.journalWebOfScienceCategory | Multidisciplinary Sciences | - |
dc.relation.journalResearchArea | Science & Technology - Other Topics | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.subject.keywordAuthor | multidimensional spectroscopy | - |
dc.subject.keywordAuthor | correlated measurement | - |
dc.subject.keywordAuthor | rotational alignment | - |
dc.subject.keywordAuthor | Raman spectroscopy | - |
dc.subject.keywordAuthor | high-resolution spectroscopy | - |
dc.subject.keywordPlus | COHERENCE SPECTROSCOPY | - |
dc.subject.keywordPlus | ALIGNMENT SPECTROSCOPY | - |
dc.subject.keywordPlus | MULTIDIMENSIONAL NMR | - |
dc.subject.keywordPlus | CARBON-DISULFIDE | - |
dc.subject.keywordPlus | CONSTANTS | - |
dc.subject.keywordPlus | SPECTROMETER | - |
dc.subject.keywordPlus | STATES | - |
dc.subject.keywordPlus | BANDS | - |
dc.subject.keywordPlus | CS2 | - |
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