Direct diversification of unmasked quinazolin-4(3: H)-ones through orthogonal reactivity modulation
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- Direct diversification of unmasked quinazolin-4(3: H)-ones through orthogonal reactivity modulation
- Lee, Jae Bin; Kang, Mi Eun; Kim, Joohee; Lee, Chang Young; Kee, Jung-Min; Myung, Kyungjae; Park, Jang-Ung; Hong, Sung You
- Issue Date
- ROYAL SOC CHEMISTRY
- CHEMICAL COMMUNICATIONS, v.53, no.75, pp.10394 - 10397
- Here we report a set of direct functionalization methods of unmasked 2-phenylquinazolin-4(3H)-ones, a privileged alkaloid core, without the installation/removal event of protecting groups or exogenous coordinating moieties. Divergent pathways were modulated with transition-metal catalysts by suppressing competitive reactivities, leading to N-arylation, annulative π-extension, or C-H fluorination.
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