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- Yang, Changduk
- Advanced Tech-Optoelectronic Materials Synthesis Lab.
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Constructing a Strongly Absorbing Low-Bandgap Polymer Acceptor for High-Performance All-Polymer Solar Cells
- Author(s)
- Zhang, Zhi-Guo, Yang, Yankang, Yao, Jia, Xue, Lingwei, Chen, Shanshan, Li, Xiaojun, Morrison, William, Yang, Changduk, Li, Yongfang
- Issued Date
- 2017-10
- Citation
- ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, v.56, no.43, pp.13503 - 13507
- Abstract
- All-polymer solar cells (all-PSCs) offer unique morphology stability for the application as flexible devices, but the lack of high-performance polymer acceptors limits their power conversion efficiency (PCE) to a value lower than those of the PSCs based on fullerene derivative or organic small molecule acceptors. We herein demonstrate a strategy to synthesize a high-performance polymer acceptor PZ1 by embedding an acceptor-donor-acceptor building block into the polymer main chain. PZ1 possesses broad absorption with a low band gap of 1.55eV and high absorption coefficient (1.3 x 10(5) cm(-1)). The all-PSCs with the wide-band-gap polymer PBDB-T as donor and PZ1 as acceptor showed a record-high PCE of 9.19% for the all-PSCs. The success of our polymerization strategy can provide a new way to develop efficient polymer acceptors for all-PSCs.
- Publisher
- WILEY-V C H VERLAG GMBH
- ISSN
- 1433-7851
- Keyword (Author)
- energy conversion, organic electronics, photoinduced force microscopy, polymers, solar cells
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