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Zhao, Bum Suk
Molecular motion control Lab.
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Strong Optical Dipole Force Exerted on Molecules Having Low Rotational Temperature

Author(s)
Sun, Xing NanJin, Byung GwunKim, Lee YeongKim, Bong JunZhao, Bum Suk
Issued Date
2016-11
DOI
10.1002/cphc.201600838
URI
https://scholarworks.unist.ac.kr/handle/201301/20664
Fulltext
http://onlinelibrary.wiley.com/doi/10.1002/cphc.201600838/full
Citation
CHEMPHYSCHEM, v.17, no.22, pp.3701 - 3708
Abstract
The optical dipole force acting on molecules is enhanced by decreasing the rotational temperature of the molecule and aligning the molecular axis with a linearly polarized nonresonant laser beam. The rotational temperature is decreased by increasing the source pressure from 2 to 81bar. By using the effective polarizability directly pertaining to the optical dipole force, the force and the resulting change in the velocity of the molecules can be evaluated. Theoretical calculations are compared with measurements based on velocity map imaging techniques. If the rotational temperature is reduced from 295 to 1K, the maximum alignment is increased from =0.33 to 0.92, and the average optical force is enhanced by 74%.
Publisher
WILEY-V C H VERLAG GMBH
ISSN
1439-4235
Keyword (Author)
cold moleculesmanipulation of moleculesmolecular alignmentmolecule opticsoptical dipole force
Keyword
ENHANCED MULTIPHOTON IONIZATIONCARBON-DISULFIDEINTENSE LIGHTLASER FIELDSBENZENELENSSTATESBEAMS

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