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Author

Song, Hyun-Kon
eclat: ElectroChemistry Lab of Advanced Technology
Research Interests
  • Electrochemical analysis, electroactive materials, electrochemistry-based energy devices

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Design of an Ultra-Durable Silicon-Based Battery Anode Material with Exceptional High-Temperature Cycling Stability

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Title
Design of an Ultra-Durable Silicon-Based Battery Anode Material with Exceptional High-Temperature Cycling Stability
Author
Park, HyungminChoi, SinhoLee, Sung-JuneCho, Yoon-GyoHwang, GaeunSong, Hyun-KonChoi, Nam-SoonPark, Soojin
Keywords
Si-based battery anodes; high-temperature cycling stability; stable solidelectrolyte-
Issue Date
201608
Publisher
Elsevier BV
Citation
NANO ENERGY, v.26, no., pp.192 - 199
Abstract
Nanostructured silicon is a promising candidate material for practical use in energy storage devices. However, high temperature operation remains a significant challenge because of severe electrochemical side reactions. Here, we show the design of ultra-durable silicon made by introducing dual coating layers on the silicon surface, allowing stable operation at high temperature. The double layers, which consist of amorphous metal titanate and carbon, provide several advantages including: (i) suppression of volume expansion during Li+ insertion; (ii) creation of a stable solid-electrolyte−interface layer; and (iii) preservation of original Si morphology over 600 cycles at high temperature. The resulting silicon-based anode exhibits a reversible capacity of 990 mAh g−1 after 500 cycles at 25 °C and 1300 mAh g−1 after 600 cycles at 60 °C with a rate of 1 C.
URI
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DOI
http://dx.doi.org/10.1016/j.nanoen.2016.05.030
ISSN
2211-2855
Appears in Collections:
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